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I can't help but think of orthogonal frequency-division multiplexing and it's use in encoding data on multiple carrier frequencies, and it makes me wonder what other parallels we will discover between digital transmission technology for cross-domain stuff like this.
Now I’m wondering what is the eigenspace of an LLM? If I take a set of LLM’s with the same number of parameters, then what are the eigenvectors? Do they have different personalities?
If it can be made orthogonal, can you go a step further and diagonalize it? The storage and performance improvement from that would be huge.
I wouldn't say that making the matrix diagonal in some basis is some further step.

If we have an singular value decomposition, M=USV^*, the columns of U are linearly independent they are a basis for the space M maps things into, and the columns of V are linearly independent then it's a basis for the space it maps things from, and [M]_{BB'} = S.

I suspect with "orthogonalization" they mean to find vectors that form an orthogonal bases (same subspace) for the vectors in the source matrix.

I wonder what would be the result if they used a matrix that is orthogonal and closest to the source matrix. Usually one uses the Frobenius norm (root of the sum of all squared matrix entries). Maybe, one could even try another norm that gives a sparser matrix.